Nitrene-Mediated Asymmetric C-H Functionalizations with Chiral Ruthenium Complexes
Transition metal catalysis is a common tool for the synthesis of enantioenriched compounds and has been well-established in organic chemistry. Nitrene chemistry, a “hot area” in recent years, has proven to be very efficient in introducing C-N bonds due to the high value of amine-containing scaffolds...
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| Format: | Doctoral Thesis |
| Language: | English |
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Philipps-Universität Marburg
2023
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| Online Access: | PDF Full Text |
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| Summary: | Transition metal catalysis is a common tool for the synthesis of enantioenriched compounds and has been well-established in organic chemistry. Nitrene chemistry, a “hot area” in recent years, has proven to be very efficient in introducing C-N bonds due to the high value of amine-containing scaffolds in various functional materials, natural products, and pharmaceuticals. This thesis presents novel catalytic asymmetric transformations mediated by a ruthenium nitrene intermediate and the synthesis as well as modification of new ruthenium complexes. |
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| Physical Description: | 262 Pages |
| DOI: | 10.17192/z2023.0653 |