Publikationsserver der Universitätsbibliothek Marburg
Titel:Methoden zur Erzeugung und Charakterisierung von geformten Femtosekunden-UV-Impulsen und deren Anwendung
Autor:Möhring, Jens
Weitere Beteiligte: Motzkus, Marcus (Prof.)
Veröffentlicht:2011
URI:https://archiv.ub.uni-marburg.de/diss/z2011/0491
URN: urn:nbn:de:hebis:04-z2011-04916
DOI: https://doi.org/10.17192/z2011.0491
DDC: Chemie
Titel (trans.):Methods for generation and characterization of shaped femtosecond UV pulses and their application
Publikationsdatum:2011-08-22
Lizenz:https://rightsstatements.org/vocab/InC-NC/1.0/

Dokument

Schlagwörter:
Ultraviolettlaser, Femtosekundenlaser, Impulsformung, Physikalische Chemie, pulse shaping, Impulslaser, Kohärente Kontrolle, coherent control, Ultraviolettspektroskopie, femtosecond laser

Zusammenfassung:
Diese Dissertation beschäftigt sich mit der Entwicklung von Methoden für die Formung und Charakterisierung von Femtosekunden-Impulsen in UV-Bereich und deren Anwendung in der zeitaufgelösten Spektroskopie. Durch Aufbau eines Impulsformers zur direkten Kontrolle von Phasen- und Amplitudenfunktion von UV-Femtosekunden-Impulsen konnte eine vielversprechende Quelle für Spektroskopie und kohärente Kontrolle entwickelt werden. Um den Einsatz geformter Impulse im UV zu unterstützen, wurden drei empfindliche Charakterisierungsmethoden für UV-Impulse im nJ-Bereich entwickelt. Dabei wurde insbesondere auch eine Impulsformer-unterstützte Methode zur referenzfreien Messung der spektralen Phase vorgestellt. Die erfolgreiche Anwendung von Femtosekunden-UV-Impulsen in der zeitaufgelösten Spektroskopie konnte am unsubstituierten Cumarin und dessen Derivat Umbelliferon (7-Hydroxy-Cumarin) demonstriert werden. Basierend auf diesen Daten wurden unter Verwendung globaler Analyseansätze Modellvorstellungen der Relaxationsdynamik in diesen Systemen entwickelt. Eine Zusammenführung von Konzepten der Femtosekunden-Impulsformung und zeitaufgelöster Spektroskopie erfolgte schließlich durch Messungen am doppelten intramolekularen Proton-Transfer von (2,2’-Bipyridyl)-3,3’-Diol oder BP(OH)2. Basierend auf diesen Daten konnten Argumente für einen rein sequentiellen Mechanismus dieser Reaktion entwickelt werden.

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